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Updating from such an old version requires careful steps to avoid "bricking" (permanently disabling) your device. How To Upgrade to PSP 6.60 PRO-C2 Custom Firmware [2021]

Upgrading a PSP from the ancient custom firmware (CFW) to modern 6.60 PRO or ME is a common task for users rediscovering their handheld consoles. While 3.52 M33 was a landmark version in the mid-2000s, it lacks support for later games, advanced plugins, and modern homebrew. Preparation: Before You Begin